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1-[(1-Methyl-1H-imidazol-2-yl)methyl]-4-phenylpiperidines as mGluR2 Positive Allosteric Modulators for the Treatment of Psychosis

Lei Zhang, Michael A. Brodney, John Candler, Angela C. Doran, Allen J. Duplantier, Ivan Efremov, E Evrard, Kenneth G. Kraus, Alan H. Ganong, Jessica Haas, Ashley N. Hanks, Keith Jenza, John T. Lazzaro, Noha Maklad, Sheryl A. Mccarthy, Weimin Qian, Bruce N. Rogers, Melinda D. Rottas, Christopher J. Schmidt, Judith A. Siuciak, F. David Tingley, Andy Q. Zhang

Journal of Medicinal Chemistry March 2, 2011 DOI: 10.1021/jm101414h via OpenAlex

Summary

AI-generated from the abstract

A new class of compounds, 1-[(1-methyl-1H-imidazol-2-yl)methyl]-4-phenylpiperidines, acts as positive allosteric modulators (PAMs) of the metabotropic glutamate receptor 2 (mGluR2). Structure-activity relationship studies produced potent and selective mGluR2 PAMs with favorable pharmacokinetic properties. The lead compound (+)-17e dose-dependently reduced methamphetamine-induced hyperactivity and mescaline-induced scratching in mice, suggesting potential for treating psychosis.

Study at a glance

Characteristics Preclinical study Peer reviewed
Population Mice
Topics Mescaline
Keywords Allosteric regulation Methamphetamine Pharmacology Allosteric modulator
Citations 32
Key finding The lead compound (+)-17e dose-dependently inhibited methamphetamine-induced hyperactivity and mescaline-induced scratching in mice.

Abstract

A novel series of mGluR2 positive allosteric modulators (PAMs), 1-[(1-methyl-1H-imidazol-2-yl)methyl]-4-phenylpiperidines, is herein disclosed. Structure-activity relationship studies led to potent, selective mGluR2 PAMs with excellent pharmacokinetic profiles. A representative lead compound (+)-17e demonstrated dose-dependent inhibition of methamphetamine-induced hyperactivity and mescaline-induced scratching in mice, providing support for potential efficacy in treating psychosis.

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